Elementary Reaction Steps in Heterogeneous Catalysis by Richard W. Joyner, Rutger A. van Santen (auth.), R. W.

By Richard W. Joyner, Rutger A. van Santen (auth.), R. W. Joyner, R. A. van Santen (eds.)

This publication contains the lawsuits of a NATO subsidized complex study Workshop held from 1st November to sixth November 1992 within the pleasant Chateau de Florans, Bedoin, Vaucluse, France and entitled 'Elementary response Steps in Heterogeneous Catalysis. ' The organisers are thankful to the technology Committee of NATO for his or her help of this assembly. this can be believed to be the 1st huge ranging NATO ARW within the box of heterogeneous catalysis for twenty years, following a prior enterprise organised in Sardinia through Basolo and Burwell, of Northwestern college, Illinois, united states [1]. This quantity collects the lecture shows and stories at the vigorous Panel discussions. the belief for the assembly advanced from a chain of overseas Symposia on Quantum Chemistry and Mechanism in Heterogeneous Catalysis. the 1st of those was once held in Lyon, France in 1986, the second one in Krakow, Poland in 1988 and the 3rd in Berkeley, California in 1990. The setting up committee of the current assembly was once Bernard Bigot, France, Tony Farragher, Netherlands, Richard Joyner, united kingdom, Mme. Danielle Olivier, France, and Rutger van Santen, Netherlands, (Chairman). we want to thank all individuals of the committee yet particularly Bernard Bigot, who undertook the very huge paintings fascinated about the neighborhood corporation with consummate ability and made our remain in Provence an excellent excitement. Bernard Bigot's secretary, Mme. Marie-Noelle Coscat and Richard Joyner's secretary, Mrs. Pat Gibbs, additionally deserve our huge thank you. there have been fifty-four contributors from 11 countries.

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J. M. Basset, J. P. Candy, A. Choplin, B. Didillon, F. Quignard and A. Theolier, in Perspectives in Catalysis J. A. Thomas, K. I. Zamaraev, Eds. (Blackwell Scientific Publications, Oxford, 1992). J. M. Basset, J. P. Candy, P. Dufour, C. Santini and A. Choplin Catalysis Today 6, I (1989). F. Hugues, J. M. Basset, Y. Ben Taarit, A. Choplin, M. Primet, D. Rojas and A. K. Smith 1. Am. Chern. Soc. 104, 7020-4 (1982). 49 6. 7. 8. 9. 10. 11. 12. 13. 14. IS. 16. 17. 18. 19. 20. 21. 22. 23. 24. 25. 26. 27.

Chem. 27,4030-3 (1988). S. B. Butts, S. H. Strauss, E. M. Holt, R. E. Stimson, N. W. Alcock and D. F. Shriver 1. Am. Chem. Soc. 102, 5093-5100 (1980). F. Quignard, C. Lecuyer, C. Bougault, F. Lefebvre, A. Choplin, D. Olivier and J. M. Basset Inorg. Chem. 31, 928-30 (1992). C. Lecuyer, F. Quignard, A. Choplin, D. Olivier and J. M. Basset Angew. Chem. Int. Ed. Engl. 30,1660-1 (1991). C. Nedez, A. Choplin, F. Lefebvre, B. Benazzi and J. M. Basset 1. Am. Chem. , accepted for publication. B. Didillon, O.

The so-called "active sites", a concept proposed by Sir H. S. Taylor [I/, may be very small in number relative to the overall surface and, consequently, their structure is almost unknown at an atomic level. It is probably this complexity which has inspired the development of surface science applied to catalysis. New concepts have emerged slowly from this approach: surface reconstruction in the presence of adsorbed molecules, surface mobility and structural reorganization of molecular-like species.

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